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The complete opposite of her sister, Chloe just wants to meet new people and to have a good time. She can often be found daydreaming or chatting on the phone.
Despite not being the twins' biological mother, Glabe Curious raised Lola and Chloe rather than their father Glarn. In fact, none of the twins has memories of him. It is possible that Glabe and Glarn were once married, but divorced and the twins were left at her care.
Unlike most alien-Sim hybrids that are the products of alien abduction, who have black hair, her hair is naturally red. It's obvious Chloe got this from her alien father, Pollination Tech#9, because he had red hair as well, as shown in the Smith family storytelling pictures.
At the start of the game Chloe has a positive but low relationship level with her twin sister, but negative daily relationships with Erin and Kristen. If free will is on, she will usually pick fights with Erin and Kristen, unless the player diverts her away from them. When the Singles household is first played, Chloe is 28 days away from becoming an elder.
As with many pre-made Sims in Strangetown, the "Skintone" part of her Sim DNA is missing.
Checking her Sim DNA in SimPE shows that she will always pass on genes for the alien skin tone, alien eyes, and red hair.
For some reason, the familial relation between the twins and Glarn's children by his second wife was left out by Maxis. This may be because the two sets of siblings have no relationships at all, and do not know one another. In any event, Chloe and Lola can marry Vidcund, Pascal, or Lazlo, their unmarried half-siblings via their human father. This can be fixed with SimPE, or the player can assume that they do not know they are related.
While the twins do not recognize Jenny as family, and don't know her, they do know her children, Jill and Johnny, and recognize them as family.
It is likely that Chloe used the Elixir of Life at least once while she was a teen. This would explain why she aged into an adult after Glabe died, while her twin became an adult before Glabe died. This could also help to explain the difference in their ages.
Her name seems to fit her, because Chloe means 'green', and Chloe is green and an alien.
She, her sister Lola, and Nervous Subject are the only living pre-made Strangetown Sims who were raised by a single parent.