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The complete opposite of her sister, Chloe just wants to meet new people and to have a good time. She can often be found daydreaming or chatting on the phone.
Despite not being the twins' biological mother, Glabe Curious raised Lola and Chloe rather than their father Glarn. In fact, none of the twins has memories of him. It is possible that Glabe and Glarn were once married, but divorced and the twins were left at her care.
Unlike most alien-Sim hybrids that are the products of alien abduction, who have black hair, her hair is naturally red. It's obvious Chloe got this from her alien father, Pollination Tech#9, because he had red hair as well, as shown in the Smith family storytelling pictures.
At the start of the game Chloe has a positive but low relationship level with her twin sister, but negative daily relationships with Erin and Kristen. If free will is on, she will usually pick fights with Erin and Kristen, unless the player diverts her away from them. When the Singles household is first played, Chloe is 28 days away from becoming an elder.
While she is technically an alien-Sim hybrid, checking her Sim DNA in SimPE shows that she will always pass on genes for the alien skin tone, alien eyes, and black hair. As a result, it is likely that any children she has will be green.
For some reason, the familial relation between Chloe and Glarn's children by his second wife was left out by Maxis. In fact, they have no relationships at all, and do not know one another. In any event, Chloe can marry Vidcund, Pascal, or Lazlo, her unmarried half-siblings via her human father. This can be fixed with SimPE, or the player can assume that they do not know they are related.
While she does not recognize Jenny as family, and does not know her, she does know Jenny's children, Jill and Johnny, and recognizes them as family.
Trivia
As with many pre-made Sims in Strangetown, the "Skintone" part of her Sim DNA is missing.
It is likely that Chloe used the Elixir of Life at least twice while she was a teen. This would explain why she aged into an adult after Glabe died, while her twin became an adult before Glabe died. This could also help to explain the difference in their ages.
Her name seems to fit her, because Chloe means 'green', and Chloe is green.
Jill and Johnny are her half-siblings and niece and nephew at the same time, as Jenny is Chloe's stepmother as well as her half-sister.
She, her sister Lola, and Nervous Subject are the only living pre-made Strangetown Sims who were raised by a single parent.